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Time-resolved photoluminescence properties of hybrids based on inorganic AlGaN/GaN quantum wells and colloidal ZnO nanocrystals

机译:基于无机AlGaN / GaN量子阱和胶体ZnO纳米晶体的杂化材料的时间分辨光致发光特性

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摘要

Dynamic properties are studied for the AlGaN/GaN quantum well (QW) structures with and without the coating of colloidal ZnO nanocrystals (NCs). The QW exciton recombination rate was reduced in such hybrids compared to the bare QW structure only in the sample with the thinnest cap layer of 3 nm. Assuming that one of the recombination mechanisms in this hybrid is non-radiative resonant energy transfer (NRET) between the QW and the energy acceptor material i.e. ZnO NCs, the maximum pumping efficiency was estimated to be similar to 42% at 60 K. The NRET effect is, however, vanished after several months despite that the hybrid structures are composed of chemically stable components. (C) 2015 Published by Elsevier Ltd.
机译:研究了具有和不具有胶体ZnO纳米晶体(NCs)涂层的AlGaN / GaN量子阱(QW)结构的动力学特性。与仅在最薄盖层为3 nm的样品中的裸QW结构相比,此类杂化物中的QW激子复合率降低。假设此混合体中的重组机制之一是QW与能量受体材料(即ZnO NCs)之间的非辐射共振能量转移(NRET),则在60 K时,最大泵浦效率估计接近42%。NRET尽管杂化结构由化学上稳定的成分组成,但几个月后这种作用消失了。 (C)2015年由Elsevier Ltd.出版

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